Time-resolved soft x-ray absorption spectroscopy of molecules in the gas and liquid phases / by Cédric Schmidt.
Schmidt, Cédric., author.
2021
QH505 .S36 2021
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Title Time-resolved soft x-ray absorption spectroscopy of molecules in the gas and liquid phases / by Cédric Schmidt.
Author Schmidt, Cédric., author.
Edition 1st ed. 2021.
ISBN 3030678385
9783030678388
3030678377
9783030678371
DOI https://doi.org/10.1007/978-3-030-67838-8.
Published Cham : Springer International Publishing, 2021.
Language English
Description 1 online resource (xvi, 119 pages, 40 illustrations, 35 illustrations in color).
Other Standard Identifiers 10.1007/978-3-030-67838-8. doi
Call Number QH505 .S36 2021
Dewey Decimal Classification 571.4
Summary This work studies the relaxation dynamics of molecules in both the gas and liquid phases after strong field ionization, using transient absorption in the soft X-rays. In particular, the thesis presents the first realization of time-resolved X-ray absorption spectroscopy in the spectral water window with a laser-based HHG source. These remarkable experiments were not only performed for isolated molecules, but also in liquids, for which the spectral coverage of the K-edges of C, N, and O are of primary importance for investigating biological molecules. The technique relies on the generation of high-order harmonics to further probe the electronic structure of molecules. Using the atomic selectivity of high energies and the temporal coherence of laser technology, we demonstrate the observation of the first stages of chemical transformation of matter in the gas and liquid phases. .
Bibliography, etc. Note Includes bibliographical references.
Access Note Access limited to authorized users.
Digital File Characteristics text file PDF
Series Springer Theses, Recognizing Outstanding Ph.D. Research, 2190-5053
In Springer Nature eBook
Available in Other Form 3-030-67837-7
Linked Resources Online Access
Record Appears in Online Resources > Ebooks
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Introduction
Theoretical Background
Method and Setup Description
Time-resolved XAS of Gas Dissociations
Pulse Peak Power Optimiza@on With Filamentation.

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