001435347 000__ 03303cam\a2200649Mi\4500 001435347 001__ 1435347 001435347 003__ OCoLC 001435347 005__ 20230309003849.0 001435347 006__ m\\\\\o\\d\\\\\\\\ 001435347 007__ cr\nn\nnnunnun 001435347 008__ 210215s2021\\\\gw\\\\\\o\\\\\000\0\eng\d 001435347 019__ $$a1237780036$$a1237863156$$a1243385687$$a1244117229$$a1249944961 001435347 020__ $$a3030678385 001435347 020__ $$a9783030678388 001435347 020__ $$z3030678377 001435347 020__ $$z9783030678371 001435347 0247_ $$a10.1007/978-3-030-67838-8.$$2doi 001435347 035__ $$aSP(OCoLC)1244123483 001435347 040__ $$aERF$$beng$$cERF$$dYDX$$dEBLCP$$dSFB$$dYDXIT$$dGW5XE$$dOCLCO$$dDCT$$dGZM$$dOCLCF$$dLEATE$$dYDX$$dUKAHL$$dOCLCO$$dOCLCQ 001435347 049__ $$aISEA 001435347 050_4 $$aQH505$$b.S36 2021 001435347 08204 $$a571.4$$223 001435347 1001_ $$aSchmidt, Cédric.,$$eauthor.$$4aut$$4http://id.loc.gov/vocabulary/relators/aut 001435347 24510 $$aTime-resolved soft x-ray absorption spectroscopy of molecules in the gas and liquid phases /$$cby Cédric Schmidt. 001435347 250__ $$a1st ed. 2021. 001435347 264_1 $$aCham :$$bSpringer International Publishing,$$c2021. 001435347 300__ $$a1 online resource (xvi, 119 pages, 40 illustrations, 35 illustrations in color). 001435347 336__ $$atext$$btxt$$2rdacontent 001435347 337__ $$acomputer$$bc$$2rdamedia 001435347 338__ $$aonline resource$$bcr$$2rdacarrier 001435347 347__ $$atext file$$bPDF$$2rda 001435347 4901_ $$aSpringer Theses, Recognizing Outstanding Ph.D. Research,$$x2190-5053 001435347 504__ $$aIncludes bibliographical references. 001435347 5050_ $$aIntroduction -- Theoretical Background -- Method and Setup Description -- Time-resolved XAS of Gas Dissociations -- Pulse Peak Power Optimiza@on With Filamentation. 001435347 506__ $$aAccess limited to authorized users. 001435347 520__ $$aThis work studies the relaxation dynamics of molecules in both the gas and liquid phases after strong field ionization, using transient absorption in the soft X-rays. In particular, the thesis presents the first realization of time-resolved X-ray absorption spectroscopy in the spectral water window with a laser-based HHG source. These remarkable experiments were not only performed for isolated molecules, but also in liquids, for which the spectral coverage of the K-edges of C, N, and O are of primary importance for investigating biological molecules. The technique relies on the generation of high-order harmonics to further probe the electronic structure of molecules. Using the atomic selectivity of high energies and the temporal coherence of laser technology, we demonstrate the observation of the first stages of chemical transformation of matter in the gas and liquid phases. . 001435347 650_0 $$aBiophysics. 001435347 650_0 $$aSpectrum analysis. 001435347 650_0 $$aMicroscopy. 001435347 650_0 $$aLasers. 001435347 650_0 $$aPhotonics. 001435347 650_0 $$aChemistry. 001435347 650_6 $$aBiophysique. 001435347 650_6 $$aMicroscopie. 001435347 650_6 $$aLasers. 001435347 650_6 $$aPhotonique. 001435347 650_6 $$aChimie. 001435347 655_0 $$aElectronic books. 001435347 7730_ $$tSpringer Nature eBook$$w(OCoLC-LEATE)288477 001435347 77608 $$z3-030-67837-7 001435347 830_0 $$aSpringer Theses, Recognizing Outstanding Ph.D. Research,$$x2190-5053 001435347 852__ $$bebk 001435347 85640 $$3Springer Nature$$uhttps://univsouthin.idm.oclc.org/login?url=https://link.springer.com/10.1007/978-3-030-67838-8$$zOnline Access$$91397441.1 001435347 909CO $$ooai:library.usi.edu:1435347$$pGLOBAL_SET 001435347 980__ $$aBIB 001435347 980__ $$aEBOOK 001435347 982__ $$aEbook 001435347 983__ $$aOnline 001435347 994__ $$a92$$bISE