TY  - GEN
AB  - Less than a decade ago, lead halide perovskite semiconductors caused a sensation: Solar cells exhibiting astonishingly high levels of efficiency. Recently, it became possible to synthesize nanocrystals of this material as well. Interestingly; simply by controlling the size and shape of these crystals, new aspects of this material literally came to light. These nanocrystals have proven to be interesting candidates for light emission. In this thesis, the recombination, dephasing and diffusion of excitons in perovskite nanocrystals is investigated using time-resolved spectroscopy. All these dynamic processes have a direct impact on the light-emitting device performance from a technology point of view. However, most importantly, the insights gained from the measurements allowed the author to modify the nanocrystals such that they emitted with an unprecedented quantum yield in the blue spectral range, resulting in the successful implementation of this material as the active layer in an LED. This represents a technological breakthrough, because efficient perovskite light emitters in this wavelength range did not exist before.
AU  - Bohn, Bernhard Johann,
CN  - QC611.8.N33
DO  - 10.1007/978-3-030-70940-2
DO  - doi
ID  - 1436730
KW  - Semiconductor nanocrystals.
KW  - Nanocrystals
KW  - Perovskite (Mineral)
KW  - Exciton theory.
KW  - Nanocristaux semi-conducteurs.
KW  - Excitons.
LK  - https://univsouthin.idm.oclc.org/login?url=https://link.springer.com/10.1007/978-3-030-70940-2
N1  - "Doctoral thesis accepted by Ludwig-Maximilians-Universität, Munich, Germany."
N2  - Less than a decade ago, lead halide perovskite semiconductors caused a sensation: Solar cells exhibiting astonishingly high levels of efficiency. Recently, it became possible to synthesize nanocrystals of this material as well. Interestingly; simply by controlling the size and shape of these crystals, new aspects of this material literally came to light. These nanocrystals have proven to be interesting candidates for light emission. In this thesis, the recombination, dephasing and diffusion of excitons in perovskite nanocrystals is investigated using time-resolved spectroscopy. All these dynamic processes have a direct impact on the light-emitting device performance from a technology point of view. However, most importantly, the insights gained from the measurements allowed the author to modify the nanocrystals such that they emitted with an unprecedented quantum yield in the blue spectral range, resulting in the successful implementation of this material as the active layer in an LED. This represents a technological breakthrough, because efficient perovskite light emitters in this wavelength range did not exist before.
SN  - 9783030709402
SN  - 303070940X
T1  - Exciton dynamics in lead halide perovskite nanocrystals :recombination, dephasing and diffusion /
TI  - Exciton dynamics in lead halide perovskite nanocrystals :recombination, dephasing and diffusion /
UR  - https://univsouthin.idm.oclc.org/login?url=https://link.springer.com/10.1007/978-3-030-70940-2
ER  -