001440519 000__ 04294cam\a2200589\i\4500 001440519 001__ 1440519 001440519 003__ OCoLC 001440519 005__ 20230309004609.0 001440519 006__ m\\\\\o\\d\\\\\\\\ 001440519 007__ cr\un\nnnunnun 001440519 008__ 211027s2021\\\\sz\a\\\\ob\\\\000\0\eng\d 001440519 019__ $$a1280602744$$a1281137645$$a1281971439$$a1287772359 001440519 020__ $$a9783030854546$$q(electronic bk.) 001440519 020__ $$a303085454X$$q(electronic bk.) 001440519 020__ $$z9783030854539 001440519 020__ $$z3030854531 001440519 0247_ $$a10.1007/978-3-030-85454-6$$2doi 001440519 035__ $$aSP(OCoLC)1280458985 001440519 040__ $$aYDX$$beng$$erda$$epn$$cYDX$$dGW5XE$$dEBLCP$$dDCT$$dOCLCF$$dOCLCO$$dOCLCQ$$dOCLCO$$dUKAHL$$dOCLCQ 001440519 049__ $$aISEA 001440519 050_4 $$aQC611.8.O7$$bA48 2021 001440519 08204 $$a537.6/226$$223 001440519 1001_ $$aAlvertis, Antonios M.,$$eauthor. 001440519 24510 $$aOn exciton-vibration and exciton-photon interactions in organic semiconductors /$$cAntonios M. Alvertis. 001440519 264_1 $$aCham :$$bSpringer,$$c[2021] 001440519 264_4 $$c©2021 001440519 300__ $$a1 online resource :$$billustrations (chiefly color) 001440519 336__ $$atext$$btxt$$2rdacontent 001440519 337__ $$acomputer$$bc$$2rdamedia 001440519 338__ $$aonline resource$$bcr$$2rdacarrier 001440519 347__ $$atext file 001440519 347__ $$bPDF 001440519 4901_ $$aSpringer theses,$$x2190-5061 001440519 500__ $$a"Doctoral thesis accepted by University of Cambridge, United Kingdom." 001440519 504__ $$aIncludes bibliographical references. 001440519 5050_ $$aIntroduction -- Organic Semiconductors and Their Properties -- The Time-Dependent Quantum Mechanical Problem -- Modelling of the Electronic and Vibrational Structure -- First Principles Modelling of Exciton-photon Interactions. 001440519 506__ $$aAccess limited to authorized users. 001440519 520__ $$aWhat are the physical mechanisms that underlie the efficient generation and transfer of energy at the nanoscale? Nature seems to know the answer to this question, having optimised the process of photosynthesis in plants over millions of years of evolution. It is conceivable that humans could mimic this process using synthetic materials, and organic semiconductors have attracted a lot of attention in this respect. Once an organic semiconductor absorbs light, bound pairs of electrons with positively charged holes, termed `excitons, are formed. Excitons behave as fundamental energy carriers, hence understanding the physics behind their efficient generation and transfer is critical to realising the potential of organic semiconductors for light-harvesting and other applications, such as LEDs and transistors. However, this problem is extremely challenging since excitons can interact very strongly with photons. Moreover, simultaneously with the exciton motion, organic molecules can vibrate in hundreds of possible ways, having a very strong effect on energy transfer. The description of these complex phenomena is often beyond the reach of standard quantum mechanical methods which rely on the assumption of weak interactions between excitons, photons and vibrations. In this thesis, Antonios Alvertis addresses this problem through the development and application of a variety of different theoretical methods to the description of these strong interactions, providing pedagogical explanations of the underlying physics. A comprehensive introduction to organic semiconductors is followed by a review of the background theory that is employed to approach the relevant research questions, and the theoretical results are presented in close connection with experiment, yielding valuable insights for experimentalists and theoreticians alike. 001440519 588__ $$aOnline resource; title from PDF title page (SpringerLink, viewed November 4, 2021). 001440519 650_0 $$aOrganic semiconductors. 001440519 650_0 $$aExciton theory. 001440519 650_6 $$aSemi-conducteurs organiques. 001440519 650_6 $$aExcitons. 001440519 655_0 $$aElectronic books. 001440519 77608 $$iPrint version:$$aAlvertis, Antonios M.$$tOn exciton-vibration and exciton-photon interactions in organic semiconductors.$$dCham : Springer, [2021]$$z3030854531$$z9783030854539$$w(OCoLC)1261303538 001440519 830_0 $$aSpringer theses,$$x2190-5061 001440519 852__ $$bebk 001440519 85640 $$3Springer Nature$$uhttps://univsouthin.idm.oclc.org/login?url=https://link.springer.com/10.1007/978-3-030-85454-6$$zOnline Access$$91397441.1 001440519 909CO $$ooai:library.usi.edu:1440519$$pGLOBAL_SET 001440519 980__ $$aBIB 001440519 980__ $$aEBOOK 001440519 982__ $$aEbook 001440519 983__ $$aOnline 001440519 994__ $$a92$$bISE