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000778965 019__ $$a968661865$$a974651041$$a981101804$$a981818549
000778965 020__ $$a9789811007736$$q(electronic book)
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000778965 0247_ $$a10.1007/978-981-10-0773-6$$2doi
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000778965 049__ $$aISEA
000778965 050_4 $$aQD281.H8
000778965 08204 $$a547/.23$$223
000778965 1001_ $$aHou, Ruijun,$$eauthor.
000778965 24510 $$aCatalytic and process study of the selective hydrogenation of acetylene and 1,3-butadiene /$$cRuijun Hou.
000778965 264_1 $$aSingapore :$$bSpringer,$$c2017.
000778965 300__ $$a1 online resource (xii, 141 pages) : color$$billustrations.
000778965 336__ $$atext$$btxt$$2rdacontent
000778965 337__ $$acomputer$$bc$$2rdamedia
000778965 338__ $$aonline resource$$bcr$$2rdacarrier
000778965 347__ $$atext file$$bPDF$$2rda
000778965 4901_ $$aSpringer theses
000778965 500__ $$a"Doctoral thesis accepted by Tsinghua University, Beijing, China."
000778965 504__ $$aIncludes bibliographical references.
000778965 5050_ $$aIntroduction -- Experimental and Theoretical Methods -- Design of Pd-Ni Bimetallic Catalyst -- Effect of Oxide Supports on Pd–Ni Bimetallic Catalysts -- Replacing Precious Metals with Carbide Catalysts -- Liquid Phase Hydrogenation of Acetylene -- Conclusion.
000778965 506__ $$aAccess limited to authorized users.
000778965 520__ $$aThis thesis offers novel methods for catalyst and process design for the selective hydrogenation of acetylene and 1,3-butadiene. The author predicts the properties of supported Pd–Ni bimetallic catalysts using density functional theory (DFT) calculations and temperature-programmed desorption (TPD). The excellent correlation between model surfaces and supported catalysts demonstrates the feasibility of designing effective bimetallic catalysts for selective hydrogenation reactions. The author also proposes a method for designing non-precious metal catalysts to replace precious metals. She modifies the process of selective hydrogenation of acetylene by coupling the selective adsorption to the selective hydrogenation in the liquid phase, as a result of which the ethylene selectivity is greatly improved and heat transfer is greatly enhanced. Lastly, by analyzing the mechanism of liquid-phase hydrogenation, the author proposes a multi-stage slurry bed reactor for industrial applications.<.
000778965 588__ $$aOnline resource; title from PDF title page (viewed February 6, 2017)
000778965 650_0 $$aHydrogenation.
000778965 650_0 $$aAcetylene.
000778965 650_0 $$aButadiene.
000778965 650_0 $$aCatalysis.
000778965 77608 $$iPrint version:$$z9789811007729
000778965 830_0 $$aSpringer theses.
000778965 852__ $$bebk
000778965 85640 $$3SpringerLink$$uhttps://univsouthin.idm.oclc.org/login?url=http://link.springer.com/10.1007/978-981-10-0773-6$$zOnline Access$$91397441.1
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