000789999 000__ 03950cam\a2200505Ii\4500 000789999 001__ 789999 000789999 005__ 20230306143331.0 000789999 006__ m\\\\\o\\d\\\\\\\\ 000789999 007__ cr\cn\nnnunnun 000789999 008__ 170622s2017\\\\gw\a\\\\ob\\\\001\0\eng\d 000789999 019__ $$a991718837$$a992537141 000789999 020__ $$a9783662552445$$q(electronic book) 000789999 020__ $$a3662552442$$q(electronic book) 000789999 020__ $$z9783662552421 000789999 020__ $$z3662552426 000789999 035__ $$aSP(OCoLC)ocn990777913 000789999 035__ $$aSP(OCoLC)990777913$$z(OCoLC)991718837$$z(OCoLC)992537141 000789999 040__ $$aN$T$$beng$$erda$$epn$$cN$T$$dEBLCP$$dN$T$$dYDX$$dGW5XE$$dOCLCF$$dUAB 000789999 049__ $$aISEA 000789999 050_4 $$aQD505 000789999 08204 $$a541.395$$223 000789999 1001_ $$aMu, Rentao,$$eauthor. 000789999 24510 $$aConstruction and reactivity of Pt-based bi-component catalytic systems /$$cRentao Mu. 000789999 264_1 $$aBerlin, Germany :$$bSpringer,$$c[2017] 000789999 300__ $$a1 online resource :$$billustrations. 000789999 336__ $$atext$$btxt$$2rdacontent 000789999 337__ $$acomputer$$bc$$2rdamedia 000789999 338__ $$aonline resource$$bcr$$2rdacarrier 000789999 4901_ $$aSpringer theses 000789999 500__ $$a"Doctoral Thesis accepted by Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian, China." 000789999 504__ $$aIncludes bibliographical references and index. 000789999 5050_ $$aSupervisors' Foreword; Parts of this thesis have been published in the following journal articles:[1] Rentao Mu, Qiang Fu*, Li Jin, Liang Yu, Guangzong Fang, Dali Tan and Xinhe Bao*, Visualizing Chemical Reactions Confined Under Graphene, Angew. Chem. Int. Ed., 2012, (51):4856-4859[2] Rentao Mu, Qiang Fu*, Hong Xu, Hui Zhang, Yuying Huang, Zhen Jiang, Shuo Zhang, Dali Tan and Xinhe Bao*, Synergetic Effect of Surface and Subsurface Ni Species at Pt-Ni Bimetallic Catalysts for CO Oxidation, J. Am. Chem. Soc., 2011, (133; Acknowledgements; Contents; 1 Introduction 000789999 5058_ $$a1.1 Modulating the Performance of Heterogeneous Catalysts1.1.1 Size Effect; 1.1.2 Surface Structure; 1.1.3 Support Effect; 1.1.4 Promotion Effect of Secondary Components; 1.2 Motivation and Conception of Thesis; References; 2 Experimental Section; 2.1 Model Samples and Precursors of Supported Nanoparticles; 2.2 UHV Systems; 2.2.1 Omicron Multi-nanoProbe System; 2.2.2 Deep Ultraviolet Photoemission Electron Microscopy System; 2.2.3 Leybold XPS System; 2.3 Experimental Methods of Model Systems; 2.4 Experimental Methods of Supported Nanoparticles; 3 Construction and Reactivity of Pt-Ni Catalysts 000789999 5058_ $$a3.1 Motivation3.2 Pt-Ni Model Catalytic Systems; 3.2.1 Preparation of Various Ni-Pt(111) Structures; 3.2.2 Interfacial Catalysis on NiO1−X/Pt(111); 3.2.3 Synergetic Effect of Surface and Subsurface Ni; 3.3 Supported Pt-Ni Nanoparticle Catalysts; 3.4 Resonable Design of Pt-Ni Bicomponent Catalysts; 3.5 Summary; References; 4 Modulating the Structure and Reactivity of Pt-Ni Catalysts; 4.1 Introduction; 4.2 Ni-Pt(111) Model Catalytic Systems; 4.3 Pt-Ni/CB Nanoparticle Catalysts; 4.4 Summary; References; 5 Comparison of Pt-Fe and Pt-Ni Catalysts; 5.1 Introduction 000789999 5058_ $$a5.2 FeOX/Pt(111) Model Catalytic Systems5.3 NiOX/Pt(111) Model Catalytic Systems; 5.4 Pt-Fe/CB and Pt-Ni/CB Nanoparticle Catalysts; 5.5 Summary; References; 6 Reactivity of Graphene-Confined Pt(111) Surface; 6.1 Introduction; 6.2 Preparation of Graphene on Pt(111) Surface; 6.3 CO Intercalation; 6.4 The Confinement Effect of Graphene; 6.5 In Situ Visualizing Single-Channel Reaction; 6.6 Summary; References; 7 Conclusions 000789999 506__ $$aAccess limited to authorized users. 000789999 588__ $$aOnline resource; title from PDF title page (viewed June 27, 2017). 000789999 650_0 $$aCatalysis. 000789999 650_0 $$aMetal catalysts. 000789999 77608 $$iPrint version:$$z9783662552421$$z3662552426$$w(OCoLC)987281990 000789999 830_0 $$aSpringer theses. 000789999 852__ $$bebk 000789999 85640 $$3SpringerLink$$uhttps://univsouthin.idm.oclc.org/login?url=http://link.springer.com/10.1007/978-3-662-55244-5$$zOnline Access$$91397441.1 000789999 909CO $$ooai:library.usi.edu:789999$$pGLOBAL_SET 000789999 980__ $$aEBOOK 000789999 980__ $$aBIB 000789999 982__ $$aEbook 000789999 983__ $$aOnline 000789999 994__ $$a92$$bISE