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Table of Contents
Intro
Supervisor's Foreword
Acknowledgements
Contents
1 Introduction
1.1 Overview
1.2 Motivation and Outline
References
2 Backgrounds
2.1 Organic Matrix-Assisted Laser Desorption Ionization (MALDI)-MS
2.2 Nanostructure-Based Laser Desorption Ionization (LDI)-MS
2.3 Research Trends in Developing LDI-Active Nanophotonic Structure
References
3 Synergistic Effect of the Hybrid of Au Nanoislands on TiO2 Nanowires (Au-TNW) in Laser Desorption and Ionization
3.1 Introduction
3.2 Experimental Methods
3.3 Results and Discussion
3.3.1 Fabrication and Characterization of Au-TNW Nanohybrid
3.3.2 LDI-MS Analysis Results of Immunosuppressive Drugs
3.3.3 Mechanistic Insights into the Synergistic Ion Production
3.4 Summary
References
4 In Situ Surface Reconstruction-Driven Desorption and Ionization Enhancement in Nanoporous Au-Modified TiO2 Nanowires Hybrid (npAu-TNW)
4.1 Introduction
4.2 Experimental Methods
4.3 Results and Discussion
4.3.1 Fabrication and Characterization of npAu-TNW Nanohybrid
4.3.2 Origin of the Enhancement in Desorption and Ionization
4.3.3 Application of npAu-TNW Nanohybrid for Neurotransmitter LDI-MS Analysis
4.4 Summary
References
5 Photothermal Structural Dynamics of Au Nanofurnace-Functionalized ZnO Nanotube (AuNI-ZNT) for In Situ Enhancement in Desorption and Ionization
5.1 Introduction
5.2 Experimental Methods
5.3 Results and Discussion
5.3.1 Fabrication and Characterization of AuNI-ZNT Nanohybrid
5.3.2 Strategies for Improving Desorption and Ionization Efficiencies
5.3.3 LDI-MS Performance Enhancement Based on AuNI-ZNT Nanohybrid
5.4 Summary
References
6 In Situ Evolution of Atomic Defect and Piezoelectricity in Graphitic Carbon Nitride Nanosheet (G-C3N4 NS) by Short Laser Pulse for the Ionization in Mass Spectrometry
6.1 Introduction
6.2 Experimental Methods
6.3 Results and Discussion
6.3.1 Fabrication and Characterization of G-C3N4 NS
6.3.2 Influence of Nanosecond Laser-Pulse-Driven Shock Pressure on LDI-MS Performance
6.3.3 G-C3N4 NS as Efficient LDI-MS Substrate
6.4 Summary
References
7 Conclusions
Supervisor's Foreword
Acknowledgements
Contents
1 Introduction
1.1 Overview
1.2 Motivation and Outline
References
2 Backgrounds
2.1 Organic Matrix-Assisted Laser Desorption Ionization (MALDI)-MS
2.2 Nanostructure-Based Laser Desorption Ionization (LDI)-MS
2.3 Research Trends in Developing LDI-Active Nanophotonic Structure
References
3 Synergistic Effect of the Hybrid of Au Nanoislands on TiO2 Nanowires (Au-TNW) in Laser Desorption and Ionization
3.1 Introduction
3.2 Experimental Methods
3.3 Results and Discussion
3.3.1 Fabrication and Characterization of Au-TNW Nanohybrid
3.3.2 LDI-MS Analysis Results of Immunosuppressive Drugs
3.3.3 Mechanistic Insights into the Synergistic Ion Production
3.4 Summary
References
4 In Situ Surface Reconstruction-Driven Desorption and Ionization Enhancement in Nanoporous Au-Modified TiO2 Nanowires Hybrid (npAu-TNW)
4.1 Introduction
4.2 Experimental Methods
4.3 Results and Discussion
4.3.1 Fabrication and Characterization of npAu-TNW Nanohybrid
4.3.2 Origin of the Enhancement in Desorption and Ionization
4.3.3 Application of npAu-TNW Nanohybrid for Neurotransmitter LDI-MS Analysis
4.4 Summary
References
5 Photothermal Structural Dynamics of Au Nanofurnace-Functionalized ZnO Nanotube (AuNI-ZNT) for In Situ Enhancement in Desorption and Ionization
5.1 Introduction
5.2 Experimental Methods
5.3 Results and Discussion
5.3.1 Fabrication and Characterization of AuNI-ZNT Nanohybrid
5.3.2 Strategies for Improving Desorption and Ionization Efficiencies
5.3.3 LDI-MS Performance Enhancement Based on AuNI-ZNT Nanohybrid
5.4 Summary
References
6 In Situ Evolution of Atomic Defect and Piezoelectricity in Graphitic Carbon Nitride Nanosheet (G-C3N4 NS) by Short Laser Pulse for the Ionization in Mass Spectrometry
6.1 Introduction
6.2 Experimental Methods
6.3 Results and Discussion
6.3.1 Fabrication and Characterization of G-C3N4 NS
6.3.2 Influence of Nanosecond Laser-Pulse-Driven Shock Pressure on LDI-MS Performance
6.3.3 G-C3N4 NS as Efficient LDI-MS Substrate
6.4 Summary
References
7 Conclusions